Two-electron ionization in strong laser fields below intensity threshold: signatures of attosecond timing in correlated spectra

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the deeply quantum regime, where the energy of the active electron driven by the laser field is insufficient to collisionally ionize the parent ion, and the assistance of the laser field is required to create a doubly charged ion. In this regime, the electron-electron and the electron-ion interactions leave distinct footprints in the correlated two-electron spectra, recording the mutual dynamics of the escaping electrons.Comment: 25 pages and 4 figure

Towards Single Atom Computing via High Harmonic Generation

The development of alternative platforms for computing has been a longstanding goal for physics, and represents a particularly pressing concern as conventional transistors approach the limit of miniaturization. A potential alternatice paradigm is that of reservoir computing, which leverages unknown, but highly non-linear transformations of input-data to perform computations. This has the advantage that many physical systems exhibit precisely the type of non-linear input-output relationships necessary for them to function as reservoirs. Consequently, the quantum effects which obstruct the further development of silicon electronics become an advantage for a reservoir computer. Here we demonstrate that even the most basic constituents of matter - atoms - can act as a reservoir for optical computers, thanks to the phenomenon of High Harmonic Generation (HHG). A prototype single-atom computer for classification problems is proposed, where parameters of the classification model are mapped to optical elements. We numerically demonstrate that this `all-optical' computer can successfully classify data with an accuracy that is strongly dependent on dynamical non-linearities. This may pave the way for the development of petahertz information processing platforms.Comment: 5 pages, 6 figure

Free to Harmonic Unitary Transformations in Quantum and Koopman Dynamics

It has long been known that there exists a coordinate transformation which exactly maps the quantum free particle to the quantum harmonic oscillator. Here we extend this result by reformulating it as a unitary operation followed by a time coordinate transformation. We demonstrate that an equivalent transformation can be performed for classical systems in the context of Koopman von-Neumann (KvN) dynamics. We further extend this mapping to dissipative evolutions in both the quantum and classical cases, and show that this mapping imparts an identical time-dependent scaling on the dissipation parameters for both types of dynamics. The derived classical procedure presents a number of opportunities to import squeezing dependent quantum procedures (such as Hamiltonian amplification) into the classical regime.Comment: 5 pages, no figure

Making Distinct Dynamical Systems Appear Spectrally Identical

We show that a laser pulse can always be found that induces a desired optical response from an arbitrary dynamical system. As illustrations, driving fields are computed to induce the same optical response from a variety of distinct systems (open and closed, quantum and classical). As a result, the observed induced dipolar spectra without detailed information on the driving field is not sufficient to characterize atomic and molecular systems. The formulation may also be applied to design materials with specified optical characteristics. These findings reveal unexplored flexibilities of nonlinear optics.Comment: 9 pages, 5 figure